ÎÒÔº³ÂÒ¶ÇàÏÈÉú2018ÄêÔÚNanoscaleÆÚ¿¯ÉϽÒÏþÁËÌâΪ¡°Concentration induced multi-color emission in carbon dots: origination from triple fluorescent centers¡±µÄÑо¿ÂÛÎÄ¡£¡£¡£¡£¡£ÂÛÎÄ×Ô½ÒÏþÒÔÀ´£¬£¬»ñµÃÁ˺£ÄÚÍâÙÉÐеĸ߶ÈÈϿɣ¬£¬²¢±»ÙÉÐжà´ÎÒýÓᣡ£¡£¡£¡£¸ÃÂÛÎÄÔÚ2019¡¢2020ÄêÁ½ÄêÁ¬ÐøÀÖ³ÉÈëÑ¡¸ß±»ÒýÂÛÎÄ!
ÂÛÎĵÄÖ÷ÒªÑо¿ÄÚÈݼ°Á¢ÒìµãÈçÏ£º£º
Ìá³öÁËŨ¶ÈÓ°ÏìµÄ¶àÉ«·¢¹â̼µã¼°ÆäÈýÖÐÐÄÓ«¹â»úÀí£º£ºÌ¼µã×÷ΪһÖÖÐÂÐ͵ÄÁãά̼ÄÉÃ×ÖÊÁÏ£¬£¬ÓÉÓÚÆä¾«²ÊµÄ¹âѧ¡¢¹âµçת»»ÐÔÄÜ£¬£¬ÔÚÉúÎï³ÉÏñ¡¢¹â´ß»¯¡¢·¢¹âÕÕÃ÷µÈÁìÓòÓÐÔ½À´Ô½¹ãµÄÓ¦Óᣡ£¡£¡£¡£µ«¹ØÓÚ̼Á¿×ÓµãµÄÔçÆÚÑо¿Ö÷Òª¼¯ÖÐÔÚÀ¶ÂÌÉ«ÇøÓò£¬£¬ÔÚ³¤²¨³¤·¢ÉäÇøÓòÑо¿Ïà¶Ô½ÏÉÙ£¬£¬²¢ÇÒȱ·¦¶Ô·¢¹â»úÀíµÄÆÊÎö¡£¡£¡£¡£¡£±¾Îı¨µÀÁËÒ»ÖÖ¶àɫӫ¹â̼µãµÄË®ÈȺϳÉÒªÁ죬£¬½ÓÄÉÄûÃÊËáÓëÒÒ´¼°·ÎªÖÊÁÏ£¬£¬Í¨¹ýµ÷ÀíÈܼÁÓë²úƷŨ¶È´Ó¶ø»ñµÃÒ»Åú¾ßÓвî±ðÓ«¹âµÄ̼µã£¬£¬·¢É䲨³¤×ª±ä´Ó450nm-600nm£¬£¬ÁýÕÖÁË´ÓÀ¶É«µ½³ÈºìÉ«ÇøÓò¡£¡£¡£¡£¡£Ñо¿Õß·¢Ã÷£¬£¬Ó«¹â·¢ÉäµÄת±äʵÖÊÉÏÔ´×ÔÓÚ̼ºË£¬£¬½çÏßÄܼ¶ºÍÍâò̬Äܼ¶ÕâÈý¸ö·¢¹âÖÐÐĵı£´æ¡£¡£¡£¡£¡£À´×ÔÓÚ¹²éîsp2¹ìµÀÔÓ»¯µÄ̼ºË²¿·Ö£¬£¬Ö÷ÒªÌåÏÖΪÀ¶É«Ó«¹â£¬£¬ÓÐËæ×ÅÒý·¢²¨³¤¸Ä±äµÄÌØÕ÷£»¶øÀ´×ÔÓÚ̼µãµÄÍâò̬Äܼ¶£¬£¬Ó«¹â²¨³¤´Ó³ÈÉ«µ½ºìÉ«£¬£¬»ù±¾²»ËæÒý·¢²¨³¤¸Ä±ä¡£¡£¡£¡£¡£Í¨¹ýÇâ¼üÁ¬ÏµµÄNÔ×ÓÔÚÆäÖÐÌåÏÖ³öÓÕµ¼Ð§Ó¦ºÍ±£»¤×÷Ó㬣¬Ê¹´ËÕ÷ÏóÔÚ¼«ÐÔ·ÇÖÊ×ÓÈܼÁÖÐÌåÏֵĸüΪÏÔ×Å£¬£¬Ò²ÎªÌ¼µãÖÊÁϵÄÓ«¹â»úÀíÑо¿ÌṩÁËÖ÷ÒªÒÀ¾Ý¡£¡£¡£¡£¡£
Ñо¿Ö°Ô±½øÒ»²½½«Ì¼µãÊèÉ¢ÓÚ»·ÑõÊ÷Ö¬ÖУ¬£¬»ñµÃÁ˾ßÓгȻÆÉ«Ó«¹âµÄ̼µã/»·ÑõÊ÷Ö¬¸´ºÏÖÊÁÏ£¬£¬¿ÉÒÔ×÷ΪLEDµÄ·â×°ÖÊÁÏ¡£¡£¡£¡£¡£Í¨¹ýµ÷Àí̼µãº¬Á¿£¬£¬¿ÉÒÔ»ñµÃů°×¹âLED£¬£¬ÆäCIE×ø±êΪ(0.42, 0.35)£¬£¬É«ÎÂΪ3100K£¬£¬Ð§ÂÊΪ14.03 lm/W¡£¡£¡£¡£¡£Òò´Ë£¬£¬ÕâÖֺϳÉÖÊÁÏÁ®¼Û¡¢ºÏ³ÉÒªÁì¼òÆÓµÄ¶àɫ̼µãÓÐÍû×÷Ϊӫ¹â·ÛµÄÌæ»»ÖÊÁÏÍÆ½ø¹âµçÆ÷¼þÌØÊâÊǰ׹âLEDÓ¦ÓõÄÀú³Ì¡£¡£¡£¡£¡£(Nanoscale, 2018, 10, 6734 - 6743)
ͼ1. (a)²î±ðŨ¶È̼µãÑùÆ·ÔÚ×ÏÍâ¹âÕÕÉäϵÄÓ«¹âÕÕÆ¬£»(b) ±ä²¨³¤Òý·¢µÄ¶þάӫ¹âͼÆ×£¬£¬Í¼ÖÐ1,2,3ÇøÓò´ú±íͬʱ±£´æÔÚA6ÑùÆ·ÖеÄÈý¸ö·¢¹âÖÐÐÄ£»(c)̼µãÈýÖÐÐÄÓ«¹â¹éÊôµÄÄ£×ÓʾÒâͼ£»(d)̼µãÑùÆ·»ìÏý»·ÑõÊ÷Ö¬·â×°LEDµÄCIE×ø±êͼºÍ(e)¹âÆ×ͼ£¬£¬²åͼΪů°×¹âLEDµÄÊÂÇéÕÕÆ¬¡£¡£¡£¡£¡£
ÂÛÎÄÈ«ÎÄÁ´½Ó£º£º
https://pubs.rsc.org/en/content/articlelanding/2018/nr/c8nr00204e#!divAbstract
ÒýÓ㺣º[1] Yeqing Chen, Hongzhou Lian, Yi Wei, Xin He, Yan Chen, Bo Wang, Qingguang Zeng,* and Jun Lin*, Concentration induced multi-color emission in carbon dots: origination from triple fluorescent centers, Nanoscale, 2018, 10, 6734-6743.